High harmonic generation from atom clusters

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چکیده

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High-order harmonic generation in atom clusters.

We report the generation of short-wavelength, high-order harmonics of intense laser radiation from atom clusters. Clusters containing about 10 3 atoms are produced in a high-pressure gas jet. We show them to be a unique nonlinear medium. Compared with monomer gases they yield a higher appearance intensity for a given harmonic order, stronger nonlinear dependence of harmonic signal on laser inte...

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Size-dependent high-order harmonic generation in rare-gas clusters.

High-order harmonic generation (HHG) is investigated in rare-gas clusters as a function of the cluster size using 0.8 and 1.3  μm femtosecond lasers. A characteristic, species-dependent knee structure in the single particle response is observed. A 1D recollision model qualitatively reproduces this behavior and associates it to the degree of delocalization of the initial wave function. Small clu...

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High-Order Harmonic Generation from Molecules

Date The final copy of this thesis has been examined by the signatories, and we find that both the content and the form meet acceptable presentation standards of scholarly work in the above mentioned discipline. High harmonic generation in atoms is well understood in terms of the three step model (ionization, propagation and recombination), and much attention has been payed to the dynamics of t...

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Enhancing and controlling single-atom high-harmonic generation spectra: a time-dependent density-functional scheme

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG spectral and temporal characteristics requires manipulating electron trajectories on attosecond time scale. The phase matching mechanism has been employed to sel...

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High-harmonic generation from an atomically thin semiconductor

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ژورنال

عنوان ژورنال: Journal of Physics: Conference Series

سال: 2014

ISSN: 1742-6588,1742-6596

DOI: 10.1088/1742-6596/508/1/012016